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Volume 37 Issue 1
Feb 2023
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Chinese Journal of High Pressure Physics  > 2023  >  37(1): 011101.
ZHANG Hongsheng, YAO Xianxiang, LYU Xindeng, SONG Hao, HUANG Yanping, FANG Yuqiang, CUI Tian. Pressure-Induced Irreversible Amorphization and Metallization of CsCu2I3[J]. Chinese Journal of High Pressure Physics, 2023, 37(1): 011101. doi: 10.11858/gywlxb.20230607
Citation: ZHANG Hongsheng, YAO Xianxiang, LYU Xindeng, SONG Hao, HUANG Yanping, FANG Yuqiang, CUI Tian. Pressure-Induced Irreversible Amorphization and Metallization of CsCu2I3[J]. Chinese Journal of High Pressure Physics, 2023, 37(1): 011101. doi: 10.11858/gywlxb.20230607
shu

Pressure-Induced Irreversible Amorphization and Metallization of CsCu2I3

doi: 10.11858/gywlxb.20230607
  • 1.

    Institute of High Pressure Physics Science, School of Physical Science and Technology, Ningbo University, Ningbo 315211, Zhejiang, China

  • 2.

    State Key Laboratory of High-Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 200050, China

  • 3.

    State Key Laboratory of Superhard Materials, College of Physics, Jilin University, Changchun 130012, Jilin, China

  • Received Date: 01 Feb 2023
  • Rev Recd Date: 05 Feb 2023
    • Available Online: 28 Feb 2023
  • Issue Publish Date: 05 Feb 2023
    Abstract
  • Exploring the structures and properties of halide perovskite under pressure have triggered great interest among scientists in recent years. However, there is still little understanding on the potential properties and applications of their amorphous phase under high pressure. In this paper, we utilized diamond anvil cell, combined with in situ high pressure synchrotron radiation X-ray diffraction, Raman spectroscopy and electrical resistance measurement to investigated the amorphization of quasi-one-dimensional halide perovskite CsCu2I3 under high pressure. It was observed that CsCu2I3 started to transform to a reversible low-density amorphous phase Ⅰ above 35.9 GPa. An irreversible high density amorphous phase Ⅱ was realized at higher pressure, which can be maintained to ambient pressure. With the application of pressure up to 136.0 GPa, the initially insulating CsCu2I3 transform to a metallic phase. In addition, the metallic amorphous phase Ⅱ can be preserved to at least 90.0 GPa. These results provide an important scientific basis for further exploring the potential properties and applications of amorphous perovskite.

     

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